Electron-phonon interaction in perovskite nanocrystals in fluorophosphate glass matrix
Bataev M. N. 1, Kuznetsova M. S 1, Pankin D. V. 1, Smirnov M. B. 1, Verbin S. Yu. 1, Ignatiev I.V. 1, Eliseyev I. A. 2, Davydov V. Yu. 2, Smirnov A. N. 2, Kolobkova E. V. 3,4
1St. Petersburg State University, St. Petersburg, Russia
2Ioffe Institute, St. Petersburg, Russia
3ITMO University, St. Petersburg, Russia
4Saint-Petersburg State Institute of Technology (Technical University), St. Petersburg, Russia
Email: batae1996@gmail.com, mashakuznecova@bk.ru, dima-pankin@mail.ru, smirnomb@rambler.ru, s.verbin@spbu.ru, i.ignatiev@spbu.ru, ilya.eliseyev@mail.ioffe.ru, valery.davydov@mail.ioffe.ru, alex.smirnov@mail.ioffe.ru, kolobok106@rambler.ru

PDF
The photoluminescence (PL) spectra of CsPbBr3 perovskite nanocrystals grown in a fluorophosphate glass matrix exhibit phonon replicas of the exciton line. The dependence of intensity of the phonon replica on its number is simulated taking into account the difference in the curvature of the excited and ground adiabatic potentials. The Raman spectra of CsPbBr3 nanocrystals are measured. Calculations based on the density functional theory is performed to obtain the spectrum of phonon states of these crystals in the orthorhombic phase. The phonon frequencies observed in the PL and Raman spectra are compared with the calculation results. Keywords: perovskites, nanocrystals, Raman scattering, phonon replicas, CsPbBr3, fluorophosphate glass.
  1. L. Protesescu, S. Yakunin, M.I. Bodnarchuk, F. Krieg, R Caputo, C.H. Hendon, R.X. Yang, A. Walsh, M.V. Kovalenko. Nano Lett., 15 (6), 3692 (2015)
  2. P. Ramasamy, D.-H. Lim, B. Kim, S.-H. Lee, M.-S. Lee, J.-S. Lee. Chem. Commun., 52, 2067 (2016)
  3. X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, H. Zeng. Advanced Functional Mater., 26 (15), 2435 (2016)
  4. M.A. Becker, R. Vaxenburg, G. Nedelcu, P.C. Sercel, A. Shabaev, M.J. Mehl, J.G. Michopoulos, S.G. Lambrakos, N. Bernstein, J.L. Lyons, T. Stoferle, R.F. Mahrt, M.V. Kovalenko, D.J. Norris, G. Raino, A.L. Efros. Nature, 553, 189 (2018)
  5. P. Li, C. Hu, L. Zhou, J. Jiang, Y. Cheng, M. He, X. Liang, W. Xiang. Mater. Lett., 209 (C), 483 (2017)
  6. S. Liu, Y. Luo, M. He, X. Liang, W. Xiang. J. Eur. Ceramic Soc., 38 (4), 1998 (2018)
  7. Y. Ye, W. Zhang, Z. Zhao, J. Wang, C. Liu, Z. Deng, X. Zhao, J. Han. Adv. Opt. Mater., 7 (9), 1801663 (2019)
  8. E. Kolobkova, M. Kuznetsova, N. Nikonorov. J. Non-Cryst. Sol., 563, 120811 (2021)
  9. A.O. Murzin, N.I. Selivanov, V.O. Kozlov, I.I. Ryzhov, T. Miyasaka, A.V. Emeline, Y.V. Kapitonov. Adv. Opt. Mater., 9 (18), 2001327 (2021)
  10. T. Yamada, T. Handa, Y. Yamada, Y. Kanemitsu. J. Phys. D: Appl. Phys., 54 (38), 383001 (2021)
  11. S. Liu, A.R. DeFilippo, M. Balasubramania n, Z. Liu, S.G. Wang, Y.-S. Chen, S. Chariton, V. Prakapenka, X. Luo, L. Zhao, J.S. Martin, Y. Lin, Y. Yan, S.K. Ghose, T.A. Tyson. Adv. Sci., 8 (18), 2003046 (2021)
  12. R. Brakkee, R.M. Williams. Appl. Sci., 10 (9), 3061 (2020)
  13. V.V. Belykh, M.L. Skorikov, E.V. Kulebyakina, E.V. Kolobkova, M.S. Kuznetsova, M.M. Glazov, D.R. Yakovlev. Nano Lett., 22 (11), 4583 (2022)
  14. X. Ma, F. Pan, H. Li, P. Shen, C. Ma, L. Zhang, H. Niu, Y. Zhu, S. Xu, H. Ye. J. Phys. Chem. Lett., 10 (20), 5989 (2019)
  15. A. Granados del'Aguila, T.T.H. Do, J. Xing, J.J. Wen, J.B. Khurgin, Q. Xiong. Nano Res., 13, 1962 (2020)
  16. W. Zhang, Y. Ye, C. Liu, J. Wang, J. Ruan, X. Zhao, J. Han. Adv. Opt. Mater., 9 (6), 2001885 (2021)
  17. M.N. Kuznetsova, Maria S. and Bataev, M.A. Chukeev, N.D. Rostovtsev, S.Y. Verbin, I.V. Ignatiev, V.Y. Davydov, A.N. Smirnov, I.A. Eliseev, E.V. Kolobkova. Opt. Spectrosc., 130 (11), 1472 (2022)
  18. S. Strohmair, A. Dey, Y. Tong, L. Polavarapu, B.J. Bohn, J.Feld-mann. Nano Lett., 20 (7), 4724 (2020)
  19. M.J. Crane, L.M. Jacoby, T.A. Cohen, Y. Huang, C.K. Luscombe, D.R. Gamelin. Nano Lett., 20 (12), 8626 (2020)
  20. P.S. Grigoryev, V.V. Belykh, D.R. Yakovlev, E. Lhuillier, M. Bayer. Nano Lett., 21 (19), 8481 (2021)
  21. E. Kirstein, N.E. Kopteva, D.R. Yakovlev, E.A. Zhukov, E.V. Kolobkova, M.S. Kuznetsova, V.V. Belykh, I.A. Yugova, M.M. Glazov, M. Bayer, A. Greilich. Nature Commun., 14 (699) (2023)
  22. R. Saran, A. Heuer-Jungemann, A.G. Kanaras, R.J. Curry. Adv. Opt. Mater., 5 (17), 1700231 (2017)
  23. Y. Guo, O. Yaffe, T.D. Hull, J.S. Owen, D.R. Reichman, L.E. Brus. Nature Commun., 10 (1), 1175 (2019)
  24. Y. Yamada, Y. Kanemitsu. NPG Asia Mater., 14 (1), 48 (2022)
  25. K. Cho, H. Tahara, T. Yamada, H. Suzuura, T. Tadano, R. Sato, M. Saruyama, H. Hirori, T. Teranishi, Y. Kanemitsu. Nano Lett., 22 (18), 7674 (2022)
  26. C.M. Iaru, A. Brodu, N.J.J. van Hoof, S.E.T. ter Huurne, J. Buhot, F. Montanarella, S. Buhbut, P.C.M. Christianen, D. Vanmaekelbergh, C. de Mello Donega, J.G. Rivas, P.M. Koenraad, A.Yu. Silov. Nature Commun., 12 (1), 5844 (2021)
  27. S.J. Clark, M.D. Segall, C.J. Pickard, P.J. Hasnip, M.I.J. Probert, K. Refson, M.C. Payne. Zeitschriftf'ur Kristallogr. --- Crystalline Mater., 220 (5-6), 567 (2005)
  28. K. Refson, P.R. Tulip, S.J. Clark. Phys. Rev. B, 73, 155114 (2006)
  29. X. Gonze, C. Lee. Phys. Rev. B, 55, 10355 (1997)
  30. J. Franck, E.G. Dymond. Trans. Faraday Soc., 21, 536 (1926)
  31. E. Condon. Phys. Rev., 28, 1182 (1926)
  32. P. Atkins. Molecular quantum mechanics (Oxford Univ. Press, Oxford, 2005)
  33. L.D. Landau, L.M. Lifshitz. Quantum Mechanics Non-Relativistic Theory. 3rd edn (Pergamon Press Ltd, 1965) v. 3, 67
  34. K. Huang, A. Rhys, N.F. Mott. Proc. Royal Society of London. Ser. A. Math. Phys. Sci., 204 (1078), 406 (1950)
  35. V.S. Krivobok, S.N. Nikolaev, V.S. Bagaev, S.I. Chentsov, E.E. Onishchenko, A.A. Pruchkina. JETP Lett., 114 (2), 98 (2021)
  36. M. Szafranski, A. Katrusiak, K. St hl. J. Mater. Chem. A, 9, 10769 (2021)
  37. C.M. Iaru, J.J. Geuchies, P.M. Koenraad, D. Vanmaekelbergh, A.Y. Silov. ACS Nano, 11 (11), 11024 (2017)
  38. X. Zhou, Z. Zhang. AIP Advances, 10 (12), 125015 (2020).

Подсчитывается количество просмотров абстрактов ("html" на диаграммах) и полных версий статей ("pdf"). Просмотры с одинаковых IP-адресов засчитываются, если происходят с интервалом не менее 2-х часов.

Дата начала обработки статистических данных - 27 января 2016 г.

Publisher:

Ioffe Institute

Institute Officers:

Director: Sergei V. Ivanov

Contact us:

26 Polytekhnicheskaya, Saint Petersburg 194021, Russian Federation
Fax: +7 (812) 297 1017
Phone: +7 (812) 297 2245
E-mail: post@mail.ioffe.ru