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New scintillation ceramics for the X-ray, γ- and neutron radiation detectors
Russian version
M.V. Korzhik1,2, V.M. Retivov2, V.V. Dubov2, L.V. Ermakova2, V.K. Ivanov3, P.V. Karpyuk2, I.A. Lagutsky4, O.Yu. Koval2, I.Yu. Komendo2, D.E. Lelekova2, V.A. Mechinsky1,2, V.A. Pustovarov5, V.G. Smyslova2, P.S. Sokolov2, D.N. Tavrunov5, A.A. Fedorov1,2
1Institute for Nuclear Problems, Belarusian State University, Minsk, Belarus
2National Research Center “Kurchatov Institute”, Moscow, Russia
3Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences, Moscow, Russia
4JSC ATOMTEX, Minsk, Belarus
5Ural Federal University after the first President of Russia B.N. Yeltsin, Yekaterinburg, Russia
Email: korjik1064@tut.by
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Methods of fabrication and scintillation properties of transparent ceramics of a garnet structure type with a composition of (Gd,Me)3Al2Ga3O12 (Me = Y,Lu), activated by ions of rare earth elements Ce, Pr, Tb. It is shown that the introduction of a compositional disorder into the cationic sublattice of compounds can significantly improve their scintillation properties. Cumulatively, in terms of their parameters the scintillators (Gd,Y)3Al2Ga3O12:Ce,Tb and (Gd,Y)3Al2Ga3O12:Ce,Pr exceed Gd2O2S:Tb,Ce, (Y,Gd)2O2S:Pr and CsI:Tl for use in the computer tomographic scanners and X-ray scanners. The scintillators (Gd,Y,Lu)3Al2Ga3O12:Ce,Mg provide a temporal resolution in matching of the annihilation γ-quanta (511 keV) below 100 ps, which makes them useful for the development of positron-emission tomographs with a possibility of additional selection during the mission. The presence of Gd ions in compounds makes it possible to create neutron counters with detector elements both, as composites and in the form of transparent elements for detecting neutrons in a wide range of the spectrum: from thermal to tens of MeV using both, the amplitude selection and the pulse shape discrimination. Keywords: scintillator, transparent ceramics, garnet, scintillations yield, X-ray scanner, positron-emission tomograph, neutron, rare-earth ions.
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