Doroshenko M. E. 1, Pierpoint K. A. 1, Jelínková H. 2, Říha A.2
1Prokhorov General Physics Institute of the Russian Academy of Sciences, Moscow, Russia
2Czech Technical University, Prague, Czech Republic
Email: pierpoint@lst.gpi.ru
The temperature dependence of the spectroscopic properties of Cr2+ ions in Zn1-xMnxSe solid solution crystals with varying manganese ion content (x=0, 0.05, and 0.3), was studied over a temperature range from 77 to 380 K. It was found that as the temperature increases, the maxima of the absorption (5T2->5E) and luminescence (5E->5T2) spectra of Cr2+ ions shift to shorter wavelengths almost linearly, at a rate of approximately 0.3 nm/K. The width of the absorption and luminescence lines increases at a rate of about 0.2 nm/K. For the crystal with x = 0.05, the lifetime of Cr2+ ions remains virtually independent of temperature up to 300 K (tau~5.5 μs) and decreases to 2.1 μs at 380 K. In the crystal with manganese content x=0.3, the lifetime is stable (tau~ 5.2 μs) up to 250 K and then drops to approximately 1.1 μs at 380 K. Keywords: Zn1-xMnxSe solid solution, Cr2+ ions, spectroscopy, temperature dependence.
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