Physics of the Solid State
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Friction-induced polarization dynamics in Bi4Ti3O12 thin films
Mishina E. D.1, Bilyk V. R.2, Sherstyuk N. E.1, Mukhortov V. M.3, Sharanov K. P.1, Agranat M.B.4, Ovchinnikov A. V.4, Sigov A. S.1
1MIREA - Russian Technological University, Moscow, Russia
2Radboud University, Nijmegen, The Netherlands
3Federal Research Center Southern Scientific Center of the Russian Academy of Sciences, Rostov-on-Don, Russia
4Joint Institute for High Temperatures, Russian Academy of Sciences, Moscow, Russia
Email: sharanov@mirea.ru

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The results of an experimental study by the method of terahertz pumping - nonlinear optical sensing of the picosecond dynamics of ferroelectric polarization induced by the action of a terahertz pulse in a ferroelectric film Bi4Ti3O12 on a silicon substrate in a wide range of the electric field strength of a THz pulse are presented. Numerical modeling based on the Landau-Khalatnikov equation of the dependences of the intensity of the second optical harmonic on the electric field shows the presence of a threshold THz field with an amplitude of Eth=4.5 MV/cm. It is shown that for small fields E<Eth, the polarization fluctuates within a certain minimum of the two-minimum potential, although in time the second harmonic signal follows the terahertz pulse. At E>Eth, polarization is switched and the time dependence of the intensity of the second harmonic becomes more complicated. Based on a comparison of theoretical and experimental data, the conditions for switching polarization by a strong electric field of a picosecond HZ pulse are analyzed. Keywords: ultrafast dynamics, polarization switching, terahertz radiation, ferroelectric films, bismuth titanate, second harmonic generation.
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