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Electron spin resonance of NV(-)-centers in synthetic fluorescent diamond microcrystals under conditions of optical spin polarization
Russian version
DOI: 10.21883/EOS.2022.12.55255.4248-22
Osipov V.Yu. 1, Bogdanov K. V. 2, Rampersaud A.3, Takai K. 4, Ishiguro Y. 5, Baranov A.V. 2
1Ioffe Institute, St. Petersburg, Russia
2ITMO University, St. Petersburg, Russia
3Columbus Nanoworks, Columbus, Ohio, United States
4Department of Chemical Science and Technology, Hosei University, Koganei, Tokyo, Japan
5Department of Electrical and Electronic Engineering, Tokyo Denki University, Tokyo, Japan
Email: osipov@mail.ioffe.ru, kirw.bog@gmail.com, arfaan@columbusnanoworks.com, takai@hosei.ac.jp, ishiguroy@mail.dendai.ac.jp, a_v_baranov@yahoo.com
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Electron paramagnetic resonance (EPR) spectra of synthetic diamond microcrystals with NV(-)-centers have been studied. It is shown that under the conditions of irradiation of the material with the light of a xenon lamp at low temperatures ~ 100 K, the intensities of the EPR signals corresponding to the "forbidden" (Delta ms=2) and low field allowed (Delta ms=1) transitions are amplified several times, while the EPR signals from paramagnetic nitrogen and impurity nickel in the charge state -1 practically do not change. This is due to a change in the population of levels of the ground triplet state of the NV(-)- center and the optical polarization of spins in the state ms=0 of the triplet level. Keywords: nitrogen-vacancy centers, synthetic diamond, electron paramagnetic resonance, spin polarization, luminescence.
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