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The vibrational-rotational high-resolution spectrum in the region of 3ν4, ν2+2ν4 and 2ν2+ν4 bands of the 72GeH4 molecule
Russian version
DOI: 10.21883/EOS.2022.03.53554.2775-21
Kuznetsov A. V.1, Raspopova N. I. 1, Gromova O. V.1, Bekhtereva E. S. 1, Koshelev M. A.2, Velmuzhova I. A3
1Tomsk Polytechnic University, Tomsk, Russia
2Institute of Applied Physics, Russian Academy of Sciences, Nizhny Novgorod, Russia
3Devyatykh Institute of Chemistry of High-Purity Substances, Russian Academy of Sciences, Nizhny Novgorod, Russia
Email: avk93@tpu.ru
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The high-resolution spectrum of the 72GeH4 molecule was recorded on a Bruker IFS 125HR Fourier spectrometer with an optical resolution of 0.003 cm-1. The line positions were analyzed for ten interacting vibrational-rotational bands 3ν4 (1F2, F1, 2F2), ν2+ 2ν4 (1E, F1, F2, 2E) and 2ν2+ν4 (1F2, F1, 2F2) in the range 2350-2750 cm-1. As a result of the analysis, 1726 experimental lines were identified with the maximum value of the quantum number Jmax = 17; then used in the fitting procedure with parameters of the effective Hamiltonian. The resulting set of 35 spectroscopic parameters describes the vibrational-rotational structure of the spectrum with drms = 7.5· 10-4 cm-1. Keywords: GeH4, spectroscopic parameters, vibrational spectrum analysis, high-resolution Fourier spectra.
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