Physics of the Solid State

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Structure, microstructure, dielectric and piezoelectric properties of solid solution ceramics of a six-component system (1-y-a-z)(Na_0.5K_0.5NbO_3)-yLiNbO_3-a/2CdNb₂O_6- zPb(Zr_0.5Ti_0.5)O₃

Russian version

Andryushin K. P.^1,2, Glazunova E. V.¹, L.A. ShilkinaL. A.¹, NagaenkoA. V.³, DudkinaS. I.¹, Andryushina I. N.¹, Khasbulatov S. V.^2,4, Reznichenko L. A.¹

¹Southern Federal University, Research Institute of Physics, Rostov-on-Don, Russia
²Kh. Ibragimov Complex Institute of the Russian Academy of Sciences, Groznyi, Russia
³Southern Federal University, Institute of High Technology and Piezo Technology, Rostov-on-Don, Russia
⁴A.A. Kadyrov Chechen State University, Institute of Mathematics, Physics and Information Technology, Grozny, Russia

Email: kpandryushin@gmail.com

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Abstract
References
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For the first time, solid solutions of two sections of a six-component system KNN-LN-PZT-CdNbO₆ of the form (1-y-a-z)(Na_0.5K_0.5NbO_3)-yLiNbO_3-a/2CdNb₂O_6-zPb(Zr_0.5Ti_0.5)O₃: were prepared by two-stage solid-phase synthesis followed by sintering using conventional ceramic technology: section I with y=0.05, a=0.025, 0.15≤ z < 0.50; section II with y =0.10, a=0.050, 0.15≤ z <0.50. X-ray diffraction revealed that all the studied experimental samples have pseudocubic symmetry. The microstructure of ceramic solid solutions is characterized by extreme inhomogeneity. An analysis of the dielectric, piezoelectric, and elastic properties (macroresponses) of the experimental samples allowed for the identification of a group of compositions with high relative permittivity values, which are promising for low-frequency applications. A conclusion is made about the feasibility of utilizing the proposed compositions in the design of electronic devices. Keywords: lead-free, (Na,K)NbO₃, CdNb₂O₆, LiNbO₃, ceramic.

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