Phase composition, crystal structure, dielectric and ferroelectric properties of Ba2NdFeNb4O15 thin films grown on a Si(001) substrate in an oxygen atmosphere
Pavlenko A. V.
1, Ilyina T. S.
1,2, Kiselev D. A.
2, Stryukov D. V.
11Federal Research Center Southern Scientific Center of the Russian Academy of Sciences, Rostov-on-Don, Russia
2National University of Science and Technology MISiS, Moscow, Russia
Email: antvpr@mail.ru, Antvpr@mail.ru, dm.kiselev@gmail.com, strdl@mail.ru
The phase composition, nanostructure, and properties of Ba2NdFeNb4O15/Si(001) multiferroic thin films have been studied by X-ray diffraction analysis, scanning probe microscopy, and capacitance-voltage characteristics analysis. The RF cathode sputtering in an oxygen atmosphere was used for films fabrication. It has been found that the obtained Ba2NdFeNb4O15 films are single-phase, impurity-free, polycrystalline textured (c-oriented), and the out-of-plane strain is 0.8%, which leads to the presence of ferroelectric properties at room temperature. It is shown that the surface roughness of the films is ~ 15.39 nm, the lateral size of the crystallites is ~ 134 nm, and the relative permittivity in the temperature range of -190...150oC is 95-130. The reasons for the revealed regularities are discussed Keywords: multiferroic, dielectric characteristics, ferroelectric, tetragonal tungsten bronze.
- Yu.S. Kuzminov. Ferroelectric crystals to control laser radiation. Nauka, M. (1982). 400 p. (in Russian)
- A.V. Pavlenko, S.P. Zinchenko, D.V. Stryukov, A.P. Kovtun, Nanorazmernye plenki niobata bariya-strontsiya: osobennosti polucheniya v plazme vysokochasotnogo razryada, struktura i fizicheskie svoistva, Izd-vo YuNTs RAN Rostov n/D (2022), 244 p. (in Russian)
- T. Hajlaoui, C. Harnagea, A. Pignolet. Mater. Lett. 198, 136 (2017)
- R. Bodeux, D. Michau, M. Josse, M. Maglione. Solid State Sci. 38, 112 (2014)
- E. Castel, P. Veber, M. Albino, M. Velazquez, S. Pechev, D. Denux, J.P. Chaminade, M. Maglione, M. Josse. J. Cryst. Growth 340, 156 (2012)
- M. Albino, P. Veber, S. Pechev, C. Labrugere, M. Velazquez, M. Maglione, M. Josse. Cryst. Growth Des. 14, 2, 500 (2014)
- V.M. Mukhortov, Yu.I. Yuzyuk, Geterostruktury na osnove nanorazmernykh segnetoelektricheskikh plyonok: poluchenie, svoistva i primenenie, YuNTs RAN, Rostov n/D (2008), 224 p. (in Russian)
- T. Hajlaoui, C. Harnagea, D. Michau, M. Josse, A. Pignolet. J. Alloys Comp. 711, 480 (2017)
- R. Bodeux, D. Michau, M. Maglione, M. Josse. Mater. Res. Bull. 81, 49 (2016)
- A.V. Pavlenko, T.S. Ilina, D.A. Kiselev, D.V. Stryukov, M.V. Ochkurov, FTT 64, 6, 658 (2022). (in Russian). DOI: 10.21883/FTT.2022.06.52391.286
- A.V. Pavlenko, D.V. Stryukov, K.M. Zhidel, Ya.Yu. Matyash, Neorgan. materialy 58, 10, 1087 (2022). (in Russian)
- R.C. Munoz, G. Vidal, M. Mulsow, J.G. Lisoni, C. Arenas, A. Concha, R. Esparza. Phys. Rev. B 62, 7, 4686 (2000)
- A.V. Pavlenko, D.A. Kiselev, Ya.Yu. Matyash, FTT 63, 6, 776 (2021)
- J.J. Zhang, J. Sun, X.J. Zheng. Solid-State Electron. 53, 170 (2009)
- L.S. Berman, FTT 35, 2, 200 (2001). (in Russian)
- A.V. Pavlenko, D.V. Stryukov. Ferroelectrics 590, 1, 220 (2022). https://doi.org/10.1080/00150193.2022.2037974
Подсчитывается количество просмотров абстрактов ("html" на диаграммах) и полных версий статей ("pdf"). Просмотры с одинаковых IP-адресов засчитываются, если происходят с интервалом не менее 2-х часов.
Дата начала обработки статистических данных - 27 января 2016 г.