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VUV 5d-4f luminescence of Gd³⁺ and Lu³⁺ ions in the CaF₂ host

Makhov V.N.^1,2, Batygov S.Kh.³, Dmitruk L.N.³, Kirm M.², Vielhauer S.², Stryganyuk G.⁴

¹P.N. Lebedev Physical Institute, Russian Academy of Sciences, Moscow, Russia

²Institute of Physics, University of Tartu, Tartu, Estonia

³General Physics Institute, Russian Academy of Sciences, Moscow, Russia
⁴Hamburger Synchrotronstrahlungslabor HASYLAB, Deutsches Elektronensynchrotron DESY, Hamburg, Germany

Email: makhov@sci.lebedev.ru

Выставление онлайн: 20 августа 2008 г.

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First observation and characterization of Lu³⁺ 4f¹³5d-4f¹⁴ luminescence from the CaF₂ : Lu³⁺ crystal are reported, and the multi-site structure in the spectra of Ce³⁺, Gd³⁺ and Lu³⁺ ions in the CaF₂ host is analyzed with the high-resolution VUV spectroscopy technique using synchrotron radiation. It was shown that vibronic structure in the emission and excitation spectra of interconfigurational transitions in Gd³⁺ and Lu³⁺ ions doped into CaF₂ differs from that observed for Ce³⁺ ions entering mainly at the tetragonal (C_4v) sites. However, the exact types of sites in which the Gd³⁺ and Lu³⁺ ions reside in the CaF₂ lattice cannot be identified basing only on obtained experimental spectroscopic data. This work was supported by the RFBR Grant 05-02-1730, the Estonian Science Foundation Grant 6538 and the European Community Research Infrastructure Action within the FP6 Program through the Contract RII3-CT-2004-506008 (IA-SFS). PACS: 78.55.Hx, 71.70.Ch, 63.20.Kr, 78.47.+p

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